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沈丽娟 教授

发布时间:2021-08-24浏览次数:6359

一、个人简介

沈丽娟,教授,博士生导师,20232024年连续入选“全球前2%顶尖科学家”榜单。福建省“杰出青年”基金获得者,主要研究方向为环境中典型有害气体的脱除和利用,聚焦H2SCO2等气体的资源转化,近年来以“材料开发-配套技术-反应创新”为主线开展系统研究,取得一系列重要进展。以第一/通讯作者在Adv. Funct. Mater., ACS Catal., Appl. Catal. B-Environ.J. Hazard. Mater.等高水平刊物上发表论文50余篇,SCI他引累计超过5000次,授权专利20余件,其中脱硫催化剂研究实现成果转化和应用。承担国家自然科学基金,国家重点研发计划子课题和福建省自然科学基金等项目。指导多名研究生获得国家奖学金、本科生荣获校级优秀毕业论文。

二、研究方向

1富含结构性碱中心材料的设计合成及其在硫化物的脱除及资源化应用;

2新型纳米材料的调控制备及其在水解制氢和有机物选择性转化的应用。

三、科研项目

1、国家自然科学基金面上项目(221780572022.01-2025.12

2、国家重点研发计划项目(2018YFA02093042018.06-2023.05

3、国家自然科学基金青年项目(216030342017.01-2019.12

4、福建省自然科学基金项目(杰青),(2024J0100262024.11-2027.11

5、福建省自然科学基金项目(2021J011972021.11-2024.11

6、福建省自然科学基金项目(2017J050222017.04-2020.04

7、校人才基金(XRC-15342015-2018


四、研究成果

代表性论文

[1] T. Shan, S. Ke, X. Yang, X. Yang, B. Weng, L. Shen*, M. Yang*,Efficient hole extraction to reactive oxidation sites over a Co3O4/Cs3Sb2Br9 p-n heterojunction for enhanced benzylic C(sp3)-H bond oxidation, Appl. Catal. B-Environ., 2025, 361, 124602.

[2] Y. Chen, S. Ke, X. Yang, L. Shen*, M. Yang*, Targeted Electron-Hole Separation to Decoupled Redox-Active Sites Over a PEA2PbBr4/CeO2 P-N Heterojunction for Enhanced Photocatalytic Oxidation, Adv. Funct. Mater.,2024, 2419519.

[3]X. Zheng, B. Li, R. Huang, W. Jiang, L. Shen*, G. Lei, S. Wang, Y. Zhan, L. Jiang*, Asymmetric Oxygen Vacancy-Promoted Synthesis of Aminoarenes from Nitroarenes Using Waste H2S as a “Hydrogen Donor”, ACS Catal.,2024, 14, 10245-10259.

[4] X. Zheng, R. Huang, B. Li, W. Jiang, L. Shen*, G. Lei, Y. Zhan*, S. Wang, L. Jiang*, Oxygen vacancies-promoted removal of COS via catalytic hydrolysis over CuTiO2-δ nanoflowers, Chem. Eng. J.,2024, 492, 152322.

[5] X. Yang, Y. Jin, S. Ke, M. Li, X. Yang, L. Shen *, M. Yang*, Cooperative S-S coupling and H2 production from photocatalytic dehydrogenation of thiols over ReSe2/ZnIn2S4 heterostructure, Chem. Eng. J.,2024, 499, 155687.

[6] L. Shen, H. Kang, L. Deng, Z. Chen, M. Yang*, Solvent-free oxidation of benzylic C(sp3)–H bond over MA3Bi2Br9 perovskite photocatalyst by efficient singlet oxygen generation, J. Catal.,2024, 434, 115499.

[7] G. Lei, Z. Yao, J. Qu, J. Chen, L. Shen *, X. Zheng, S. Wang, Y. Cao, Y. Zhan*, Modulating oxygen vacancies of Fe-doped Ti-based materials with ultrathin nanosheets for enhancing H2S-to-S selective oxidation, Chem. Eng. J.,2024, 485, 150007.

[8] T. Shan, Y. Li, S. Ke, B.Su, L. Shen*, S. Wang*, X. Yang, M. Yang*, An embedded ReS2@MAPbBr3 heterostructure with downhill interfacial charge transfer for photocatalytic upgrading of biomass-derived alcohols to aldehydes and H2,J. Mater. Sci. Technol.,2024, 179, 155-165.

[9] X. Zheng, X. Chen, X. Li, J. Zhu, J. Chen, F. Lin, L. Shen*, Y. Xu*, L. Jiang, Designed Synthesis of Fe/Zr Bimetallic Organic Framework to Enhance the Selective Conversion of H2S to Sulfur, Inorg. Chem.,2024, 63, 5586−5597.

[10] Y. Chen, T. Shan, L. Liu, L. Shen*, H. Xue, M. Yang*, Construction of embedded CdS nanosheets@PEA2PbBr4 nanoplate p-n heterojunction photocatalysts with spatial charge transfer for enhanced benzylic C(sp3)-H bond oxidation, Chem. Eng. J., 2024, 480, 148099.

[11] M. Li, S. Ke, X. Yang, L. Shen*, M. Yang*, S-scheme homojunction of 0D cubic/2D hexagonal ZnIn2S4 for efficient photocatalytic reduction of nitroarenes, J. Colloid Interf. Sci., 2024, 674, 547-559

[12] X. Zheng, G. Lei, S. Wang, L. Shen*, Y. Zhan, L. Jiang*, Advances in Resources Recovery of H2S: A Review of Desulfurization Processes and Catalysts, ACS Catal.,2023, 13, 11723-11752.

[13] G. Lei, Z. Fan, Y. Hou, F. Liu, S. Wang, L. Shen*, Y. Zhan, L. Jiang*, Facile template-free synthesis of 3D cluster-like nitrogen-doped mesoporous carbon as metal-free catalyst for selective oxidation of H2S, J. Environ. Chem. Eng.,2023, 11, 109095.

[14] G. Lei, S. Qi, H. Li, Y. Xue, L. Shen*, X. Zheng, S. Wang, Y. Cao, Y. Zhan*, Carbon-doped boron nitride nanosheets as an efficient metal-free catalyst for the selective oxidation of H2S, Phys. Chem. Chem. Phys., 2023, 25, 32317-32322.

[15] G. Lei, Y. Zheng, Y. Cao, L. Shen*, S. Wang, S. Liang, Y. Zhan*, L. Jiang*, Deactivation Mechanism of COS Hydrolysis over Potassium Modified Alumina,Acta Phys. Chim. Sin., 2023, 39, 2210038

[16]G. Lei, Z. Fan, Y. Hou, F. Liu, S. Wang, L. Shen*, Y. Zhan, L. Jiang*, Facile template-free synthesis of 3D cluster-like nitrogen-doped mesoporous carbon as metal-free catalyst for selective oxidation of H2S, J. Environ. Chem. Eng., 2023, 11, 109095.

[17] L. Deng, M. Li, L. Luo, T. Chen, T. Shan, X. Yang, L. Shen*, M. Yang*, In-situ construction of FAPbBr3-wrapped MoS2 heterostructure for photocatalytic H2 evolution from dehydrogenation of aromatic alcohols, Appl. Surf. Sci., 2023, 638, 158004.

[18] G. Lei, D. Li, Y. Ma, S. Wang, L. Shen*, Y. Zhan*, L. Jiang, Holey carbon nanomeshes with atomically Cu–N4 active sites for efficient carbonyl sulfide catalytic hydrolysis, Carbon, 2023, 210, 118039.

[19] T. Chen, B. Weng, S. Lu, H. Zhu, Z. Chen, L. Shen*, M. B. J. Roeffaers*, M. Yang*, Photocatalytic Anaerobic Dehydrogenation of Alcohols over Metal Halide Perovskites: A New Acid-Free Scheme for H2 Production, J. Phys. Chem. Lett.,2022, 13, 6559−6565.

[20] Y. Cao, W. You, G. Lei, X. Zheng, L. Shen*, F. Liu, L. Jiang*, Enabling High Efficiency and Rapid Regeneration of α FeOOH@Fe-EDTA for Slurry Desulfurization, Ind. Eng. Chem. Res., 2022, 61, 249−258.

[21] X. Zheng, G. Zhang, Z. Yao, Y. Zheng, L. Shen*, F. Liu, Y. Cao, S. Liang*, Y. Xiao, L. Jiang, Engineering of crystal phase over 3D porous MnO2 for highly efficient elimination of H2S, J. Hazard. Mater., 2021, 411, 125180.

[22]X. Zheng, J. Cai, Y. Cao, L. Shen*, Yong Zheng, F. Liu, S. Liang *, Y. Xiao, L. Jiang*, Construction of cross-linked δ-MnO2 with ultrathin structure for the oxidation of H2S: Structure-activity relationship and kinetics study, Appl. Catal. B-Environ., 2021, 297, 120402.

[23] G.Lei, Y. Tong, L. Shen*, Y. Zheng, S. Liang,* W. Lin, F. Liu, Y. Cao, Y. Xiao, L. Jiang*Highly Poison-Resistant Single-Atom Co–N4 Active Sites with Superior Operational Stability over 460 h for H2S Catalytic Oxidation,Small,2021, 17, 2104939.

[24] J. Cai, X. Zheng, W. You, L. Shen*, Y. Zheng, Y. Cao, Y. Xiao, L. Jiang*, Porous flake-like Al-rich MgAl2O4 endowed with Mg vacancies for efficient oxidative desulfurization, Appl. Catal. A: Gen.,2021, 623, 118238.

[25] L. Shen, G. Lei, Y. Zheng, S. Liang*, F. Liu, S. Wang*, Y. Cao, Y. Xiao, L. Jiang* Electronic Regulation of Bromophenyl Grafted Metal-Free Carbon Nitride Catalysts for Enhanced Utilization of H2S, ChemCatChem, 2021, 13, 2386-2392.

[26] X. Zheng, S. Qi, Y. Cao, L. Shen*, C. Au, L. Jiang*, Morphology evolution of acetic acid-modulated MIL-53(Fe)for efficient selective oxidation of H2S, Chinese J. Catal., 2021, 42, 279–287.

[27] X. Zheng, J. Cai, W. Zhao, S. Liang*, Y. Zheng, Y. Cao, L. Shen*, Y. Xiao, L. Jiang, Porous α-Fe2O3/SnO2 nanoflower with enhanced sulfur selectivity and stability for H2S selective oxidation, Chinese Chem. Lett., 2021, 32, 2143-2150.

[28] G. Lei, Y. Tong, L. Shen*, F. Liu, Y. Xiao, W. Lin, Y. Zhang, C. Au, L. Jiang*,Highly Active and Sulfur Resistant Fe–N4 Sites in Porous Carbon Nitride for Oxidative Desulfurization, Small, 2020, 2003904.

[29] X. Zheng, Y. Li, Y. Zheng, L. Shen*, Y. Xiao, Y. Cao, Y. Zhang, C. Au, L. Jiang*, Highly Efficient Porous FexCe1–xO2δ with Three-Dimensional Hierarchical Nanoflower Morphology for H2S-Selective Oxidation, ACS Catal., 2020, 10, 3968-3983.

[30] X. Zheng, Y. Li, S. Liang*, Z. Yao, Y. Zheng, L. Shen*, Y. Xiao, Y. Zhang, C. Au, L. Jiang*, Promoting effect of Cu-doping on catalytic activities and SO2 resistance of porous CeO2 nanorods for H2S selective oxidation, J. Catal., 2020, 389, 382-399.

[31] G. Lei, W. Zhao, L. Shen*, S. Liang, C. Au, L. Jiang*, Isolated iron sites embedded in graphitic carbon nitride (g-C3N4) for efficient oxidative desulfurization, Appl. Catal. B-Environ., 2020, 267, 118663.

[32] X. Zheng, Z. Fang, Z. Dai, J. Cai, L. Shen*, Y. Zhang, C. Au, L. Jiang*, Iron-Based Metal-Organic Frameworks as Platform for H2S Selective Conversion: Structure-Dependent Desulfurization Activity, Inorg. Chem., 2020, 59, 4483-4492.

[33] X. Zheng, Y. Li, L. Zhang, L. Shen*, Y. Xiao, Y. Zhang, C. Au, L. Jiang*, Insight into the effect of morphology on catalytic performance of porous CeO2 nanocrystals for H2S selective oxidation, Appl. Catal. B-Environ., 2019, 252, 98-110.

[34] G. Lei, Z. Dai, Z. Fan, X. Zheng, Y. Cao, L. Shen*, Y. Xiao, C. Au, L. Jiang*, Porous nanosheets of carbon-conjugated graphitic carbon nitride for the oxidation of H2S to elemental sulfur, Carbon, 2019, 155, 204-214.

[35] X. Zheng, L. Zhang, Z. Fan, Y. Cao, L. Shen*, C. Au, L. Jiang*, Enhanced catalytic activity over MIL-100(Fe) with coordinatively unsaturated Fe2+/Fe3+ sites for selective oxidation of H2S to sulfur, Chem. Eng. J., 2019, 374, 793-801.

[36] G. Lei, Y. Cao, W. Zhao, Z. Dai, L. Shen,* Y. Xiao, L. Jiang,* Exfoliation of graphitic carbon nitride for enhanced oxidative desulfurization: A facile and general strategy, ACS Sustainable Chem. Eng., 2019, 7, 4941-4950.

[37] W. Zhao, X. Zheng, S. Liang, X. Zheng, L. Shen*, F. Liu, Y. Cao, Z. Wei, L. Jiang*, Fe-doped γ-Al2O3 porous hollow microspheres for enhanced oxidative desulfurization: facile fabrication and reaction mechanism, Green Chem., 2018, 20, 4645-4654.

[38] L. Shen, X. Zheng, G. Lei, X. Li, Y. Cao, L. Jiang, Hierarchically porous γ-Al2O3 nanosheets: Facile template-free preparation and reaction mechanism for H2S selective oxidation, Chem. Eng. J., 2018, 346, 238-248.

[39] L. Shen, G. Lei, Y. Fang, Y. Cao, X. Wang, L. Jiang, Polymeric carbon nitride nanomesh as an efficient and durable metal-free catalyst for oxidative desulfurization, Chem. Commun., 2018, 54, 2475-2478.

[40] L. Shen, Y. Xia, S. Lin, S. Liang, L. Wu, An unsaturated metal site-promoted approach to construct strongly coupled noble metal/HNb3O8 nanosheets for efficient thermo/photo-catalytic reduction, Nanoscale, 2017, 9, 14654-14663.

[41] L. Shen, Y. Cao, Z. Du, W. Zhao, K. Lin, L. Jiang, Illuminate the active sites of γ-FeOOH for low-temperature desulfurization, Appl. Surf. Sci., 2017, 425, 212-219.

[42] L. Shen, G. Wang, X. Zheng, Y. Cao, Y. Guo, K. Lin, L. Jiang, Tuning the growth of Cu-MOFs for efficient catalytic hydrolysis of carbonyl sulfide, Chinese J. Catal.,2017, 38, 1373-1381.

[43] L. Shen, C. Xu, X. Qi, Y. Cao, J. Tang, Y. Zheng, L. Jiang, Highly efficient CuxO/TiO2 catalysts: controllable dispersion and isolation of metal active species, Dalton T., 2016, 45, 4491-4495.

[44] L. Shen, M. Luo, L. Huang, P. Feng, L. Wu, A Clean and General Strategy To Decorate a Titanium Metal–Organic Framework with Noble-Metal Nanoparticles for Versatile Photocatalytic Applications, Inorg. Chem.,2015, 54, 1191-1193.

[45] L. Shen, M. Luo, Y. Liu, R. Liang, F. Jing, L. Wu, Noble-metal-free MoS2 co-catalyst decorated UiO-66/CdS hybrids for efficient photocatalytic H2 production, Appl. Catal. B-Environ.,2015, 166-167, 445-453.

[46] L. Shen, R. Liang, L. Wu, Strategies for engineering metal-organic frameworks as efficient photocatalysts, Chinese J. Catal., 2015, 36, 2071-2088.

[47] L. Shen, R. Liang, M. Luo, F. Jing, L. Wu, Electronic effects of ligand substitution on metal-organic framework photocatalysts: the case study of UiO-66, Phys. Chem. Chem. Phys, 2015, 17, 117-121.

六、联系方式

电子邮箱:ljshen@fjnu.edu.cn

通讯地址:福建省福州市大学城科技路1号福建师范大学旗山校区理工6号楼环境与资源学院


常用链接

0591-22868175
福建省福州市大学城科技路1号福建师范大学旗山校区理工楼6号楼
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